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Many, if not most, step polymerizations involve equilibrium reactions, and it becomes important to analyze how the equilibrium affects the extent of conversion and, more importantly, the polymer molecular weight. A polymerization in which the monomer(s) and polymer are in equilibrium is referred to as an equilibrium polymerization or reversible polymerization. A rst consideration is whether an equilibrium polymerization will yield high-molecularweight polymer if carried out in a closed system. By a closed system is meant one where none of the products of the forward reaction are removed. Nothing is done to push or drive the equilibrium point for the reaction system toward the polymer side. Under these conditions the concentrations of products (polymer and usually a small molecule such as water) build up until the rate of the reverse reaction becomes equal to the polymerization rate. The reverse reaction is referred to generally as a depolymerization reaction; other terms such as hydrolysis or glycolysis may be used as applicable in speci c systems. The polymer molecular weight is determined by the extent to which the forward reaction has proceeded when equilibrium is established. Consider an external acid-catalyzed polyesteri cation

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Hagiwara, T, M Ishimori, and T Tsuruta, Makromol Chem, 182, 501 (1981) Hall, H K, Jr, J Amer Chem Soc, 80, 6404 (1958) Hall, H K, Jr and L G Snow, Ring-Opening Polymerization via Carbon-Carbon s-Bond Cleavage, Chap 2 in Ring-Opening Polymerization, Vol 2, K J Ivin and T Saegusa, eds, Elsevier, London, 1984 Hasebe, Y and T Tsuruta, Makromol Chem, 189, 1915 (1988) Hasegawa, E, T Shibata, H Takeuchi, and E Tsuchida, Eur Polym J, 13, 669 (1977) Hashimoto, K, Prog Polym Sci, 25, 1411 (2000) Hauser, M, Alkylenimines, Chap 5 in Ring-Opening Polymerization, K C Frisch and S L Reegen, eds, Marcel Dekker, New York, 1969 Hermans, P H, D Heikens, and P F van Velden, J Polym Sci, 30, 81 (1958); 44, 437 (1960) Herweh, J E, J Polym Sci.

Polym Chem Ed, 27, 333 (1989) Higashimura, T, A Tanaka, T Miki, and S Okamura, J Polym Sci, A-1(5), 1927, 1937 (1967) Hirasawa, T, M Okada, and H Sumitoma, Macromolecules, 21, 1566 (1988) Hirota, M and H Fukuda, Makromol Chem, 188, 2259 (1987) Hofman, A, S Slomkowski, and S Penczek, Makromol Chem, 188, 2027 (1987a); Makromol Chem Rapid Commun, 8, 387 (1987b) Hofman, A, R Szymanski, S Slomkowski, and S Penczek, Makromol Chem, 185, 655 (1985) Hoyle, C E, S F Thames, L R Mullen, and D L Schmidt, J Polym Sci Polym Chem Ed, 39, 571 (2001) Imanishi, Y, N-Carboxyanhydrides, Chap 8 in Ring-Opening Polymerization, Vol 1, K J Ivin and T Saegusa, eds, Elsevier, London, 1984 Imanishi, Y, A Aoyama, Y Hashimoto, and T Higashimura, Biopolymers, 16, 187 (1977) Inoue, S, J.

In 1773 the words the Stock Exchange were written over the door of New Jonathan s Coffee House, and admittance was permitted only by fee In 1802 the Stock Exchange built its own home Mortgages at this time did not provide, as they do today, a fixed rate of return over long periods of time Interest was variable because usually either party could withdraw from the contract on six months notice Furthermore, real estate mortgages, which were a principal form of borrowing.

Macromol Sci Chem, A25, 571 (1988); J Polym Sci Polym Chem Ed, 38, 2861 (2000) Inoue, S and T Aida, Cyclic Ethers, Chap 4 in Ring-Opening Polymerization, Vol 1, K J Ivin and T Saegusa, eds, Elsevier, London, 1984 Inoue, S and T Aida, Anionic Ring-Opening Polymerization: Copolymerization, Chap 37 in Comprehensive Polymer Science, Vol 3, G C Eastmond, A Ledwith, S Russo, and P Sigwalt, eds, Pergamon Press, London, 1989 Ishii, Y and S Sakai, 1,2-Epoxides, Chap 2 in Ring-Opening Polymerization, K C Frisch and S L Reegen, eds, Marcel Dekker, New York, 1969 Ishizu, K, S Ishikawa, and T Fukutomi, J Polym Sci Polym Chem Ed, 23, 445 (1985) IUPAC, Pure Appl Chem, 48, 375 (1976); 57, 149 (1985); 66, 2483 (1994); 74, 1921 (2002) Ivin, K J, Cycloalkenes and Bicycloalkenes, Chap 3 in Ring-Opening Polymerization, Vol 1, K.

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